Dynamics of a quantum interacting system: Extended global approach beyond the Born-Markov and secular approximation

• URL: http://arxiv.org/abs/2303.02926v2
• Date: Thu, 14 Sep 2023 01:24:45 GMT
• Title: Dynamics of a quantum interacting system: Extended global approach beyond the Born-Markov and secular approximation
• Authors: Chikako Uchiyama
• Abstract summary: We present a formalism that leads to the time-convolutionless (time-local) master equation. We apply it to the excitation energy transfer between interacting sites in which only the terminal site weakly interacts with a bosonic environment of finite temperature.
• Score: 0.0
• License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
• Abstract: In various fields from quantum physics to biology, the open quantum dynamics of a system consisting of interacting subsystems emphasizes its fundamental functionality. The local approach, deriving a dissipator in a master equation by ignoring the inter-subsystem interaction, has been widely used to describe the reduced dynamics due to its robustness to keep the positivity of a density operator. However, one critique is that a stationary state obtained by the approach in the limit of weak system-environment coupling is written in the form of the Gibbs state for the partial Hamiltonian by excluding the inter-subsystem interaction from the total one of the relevant system. As an alternative, the global approach, deriving a dissipator with including the inter-subsystem interaction, under the Born--Markov and secular approximations has attracted much attention, and there is debate concerning its violation of positivity in the short-term region and/or limited parameter region for the Bohr frequencies of the subsystems. In this study, we present a formalism that leads to the time-convolutionless (time-local) master equation obtained by extending the global approach beyond the Born-Markov and secular approximations. We apply it to the excitation energy transfer between interacting sites in which only the terminal site weakly interacts with a bosonic environment of finite temperature in a manner beyond the rotating-wave approximation. We find that the formulation (1) gives the short-time behavior while preserving positivity, (2) shows the oscillatory features that the secular approximation would obscure, and (3) leads to a stationary state very near to the Gibbs state for the total Hamiltonian of the relevant system.

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