Hybrid interfaces at the single quantum level in fluorescent molecules

• URL: http://arxiv.org/abs/2503.20872v3
• Date: Wed, 23 Apr 2025 18:00:04 GMT
• Title: Hybrid interfaces at the single quantum level in fluorescent molecules
• Authors: Daniele De Bernardis, Hugo Levy-Falk, Elena Fanella, Rocco Duquennoy, Valerio Digiorgio, Giacomo Scalari, Maja Colautti, Costanza Toninelli,
• Abstract summary: Multiple external laser sources exert control of the vibronic states of a single fluorescent molecule.<n>The steady state exhibits vibrational bi-modality resulting in a statistical mixture of non-classical vibronic cat states.<n>This work assesses the role of molecules as an optomechanical quantum toolbox for creating hybrid entangled states of electrons, photons, and vibrations.
• Score: 0.0
• License: http://creativecommons.org/licenses/by/4.0/
• Abstract: We theoretically investigate a single fluorescent molecule as a hybrid quantum optical device, in which multiple external laser sources exert control of the vibronic states. In the high-saturation regime, a coherent interaction is established between the vibrational and electronic degrees of freedom, and molecules can simulate several cavity QED models, whereby a specific vibrational mode plays the role of the cavity mode. Focusing on the specific example where the system is turned into an analogue simulator of the quantum Rabi model, the steady state exhibits vibrational bi-modality resulting in a statistical mixture of highly non-classical vibronic cat states. Applying our paradigm to molecules with prominent spatial asymmetry and combining an optical excitation with a THz(IR) driving, the system can be turned into a single photon transducer. Two possible implementations are discussed based on the coupling to a subwavelength THz patch antenna or a resonant metamaterial. In a nutshell, this work assesses the role of molecules as an optomechanical quantum toolbox for creating hybrid entangled states of electrons, photons, and vibrations, hence enabling frequency conversion over very different energy scales.

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