Twenty-three millisecond electron spin coherence of erbium ions in a
natural-abundance crystal
- URL: http://arxiv.org/abs/2106.14974v1
- Date: Mon, 28 Jun 2021 20:45:11 GMT
- Title: Twenty-three millisecond electron spin coherence of erbium ions in a
natural-abundance crystal
- Authors: Marianne Le Dantec, Milo\v{s} Ran\v{c}i\'c, Sen Lin, Eric Billaud,
Vishal Ranjan, Daniel Flanigan, Sylvain Bertaina, Thierry Chaneli\`ere,
Philippe Goldner, Andreas Erb, Ren Bao Liu, Daniel Est\`eve, Denis Vion,
Emmanuel Flurin, Patrice Bertet
- Abstract summary: This is the longest electron spin coherence time measured in a material with a natural abundance of nuclear spins.
Our results establish Er$3+$:CaWO$_4$ as a leading platform for quantum networks.
- Score: 0.8331845551768636
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: Erbium ions doped into crystals have unique properties for quantum
information processing, because of their optical transition at 1.5 $\mu$m and
of the large magnetic moment of their effective spin-1/2 electronic ground
state. Most applications of erbium require however long electron spin coherence
times, and this has so far been missing. Here, by selecting a host matrix with
a low nuclear-spin density (CaWO$_4$) and by quenching the spectral diffusion
due to residual paramagnetic impurities at millikelvin temperatures, we obtain
an Er$^{3+}$ electron spin coherence time of 23 ms. This is the longest
electron spin coherence time measured in a material with a natural abundance of
nuclear spins and on a magnetically-sensitive transition. Our results establish
Er$^{3+}$:CaWO$_4$ as a leading platform for quantum networks.
Related papers
- Coherent control of a nuclear spin via interactions with a rare-earth
ion in the solid-state [0.0]
Individually addressed Er$3+$ ions in solid-state hosts are promising resources for quantum repeaters.
While the Er$3+$ electron spin provides a spin-photon interface, ancilla nuclear spins could enable multi-qubit registers with longer storage times.
We demonstrate coherent coupling between the electron spin of a single Er$3+$ ion and a single $I=1/2$ nuclear spin in the solid-state host crystal.
arXiv Detail & Related papers (2022-09-12T21:44:21Z) - Robust millisecond coherence times of erbium electron spins [7.862622132486542]
We report GHz-range electron spin transitions of $167mathrmEr3+$ in yttrium oxide.
We find paramagnetic impurities are the dominant source of decoherence.
These coherence lifetimes are among the longest found in crystalline hosts.
arXiv Detail & Related papers (2022-07-06T14:29:11Z) - Electron spin coherence on a solid neon surface [2.5496329090462626]
A single electron floating on the surface of a condensed noble-gas liquid or solid can act as a spin qubit with ultralong coherence time.
Previous studies suggest that the electron spin coherence time on a superfluid helium (He) surface can exceed 100 s.
We present theoretical studies of the electron spin coherence on a solid neon (Ne) surface, motivated by our recent experimental realization of single-electron charge qubit on solid Ne.
arXiv Detail & Related papers (2022-05-02T00:32:25Z) - Computational Insights into Electronic Excitations, Spin-Orbit Coupling
Effects, and Spin Decoherence in Cr(IV)-based Molecular Qubits [63.18666008322476]
We provide insights into key properties of Cr(IV)-based molecules aimed at assisting chemical design of efficient molecular qubits.
We find that the sign of the uniaxial zero-field splitting (ZFS) parameter is negative for all considered molecules.
We quantify (super)hyperfine coupling to the $53$Cr nuclear spin and to the $13C and $1H nuclear spins.
arXiv Detail & Related papers (2022-05-01T01:23:10Z) - Electron-spin spectral diffusion in an erbium doped crystal at
millikelvin temperatures [0.8961088845748072]
We characterize the spectral diffusion processes that limit the electron-spin coherence of Er ions at millikelvin temperatures.
The coherence time shows a strong temperature dependence, reaching 1.3 ms at 23 mK for an electron-spin transition of $167textEr$.
arXiv Detail & Related papers (2022-03-28T18:20:47Z) - Relativistic aspects of orbital and magnetic anisotropies in the
chemical bonding and structure of lanthanide molecules [60.17174832243075]
We study the electronic and ro-vibrational states of heavy homonuclear lanthanide Er2 and Tm2 molecules by applying state-of-the-art relativistic methods.
We were able to obtain reliable spin-orbit and correlation-induced splittings between the 91 Er2 and 36 Tm2 electronic potentials dissociating to two ground-state atoms.
arXiv Detail & Related papers (2021-07-06T15:34:00Z) - Anisotropic electron-nuclear interactions in a rotating quantum spin
bath [55.41644538483948]
Spin-bath interactions are strongly anisotropic, and rapid physical rotation has long been used in solid-state nuclear magnetic resonance.
We show that the interaction between electron spins of nitrogen-vacancy centers and a bath of $13$C nuclear spins introduces decoherence into the system.
Our findings offer new insights into the use of physical rotation for quantum control with implications for quantum systems having motional and rotational degrees of freedom that are not fixed.
arXiv Detail & Related papers (2021-05-16T06:15:00Z) - Experimental Constraint on an Exotic Parity-Odd Spin- and
Velocity-Dependent Interaction with a Single Electron Spin Quantum Sensor [6.887744934296352]
Experiment set improved constraints on the exotic spin- and velocity-dependent interaction within the force range from 1 to 330 $mu$m.
The upper limit of the coupling $g_Aeg_VN $ at $200 mu m$ is $| g_Ae g_VN| leq 8.0times10-19$, significantly improving the current laboratory limit by more than four orders of magnitude.
arXiv Detail & Related papers (2020-09-19T15:31:21Z) - Electrically tuned hyperfine spectrum in neutral
Tb(II)(Cp$^{\rm{iPr5}}$)$_2$ single-molecule magnet [64.10537606150362]
Both molecular electronic and nuclear spin levels can be used as qubits.
In solid state systems with dopants, an electric field was shown to effectively change the spacing between the nuclear spin qubit levels.
This hyperfine Stark effect may be useful for applications of molecular nuclear spins for quantum computing.
arXiv Detail & Related papers (2020-07-31T01:48:57Z) - Quantum coherent spin-electric control in a molecular nanomagnet at
clock transitions [57.50861918173065]
Electrical control of spins at the nanoscale offers architectural advantages in spintronics.
Recent demonstrations of electric-field (E-field) sensitivities in molecular spin materials are tantalising.
E-field sensitivities reported so far are rather weak, prompting the question of how to design molecules with stronger spin-electric couplings.
arXiv Detail & Related papers (2020-05-03T09:27:31Z) - Hyperfine and quadrupole interactions for Dy isotopes in DyPc$_2$
molecules [77.57930329012771]
Nuclear spin levels play an important role in understanding magnetization dynamics and implementation and control of quantum bits in lanthanide-based single-molecule magnets.
We investigate the hyperfine and nuclear quadrupole interactions for $161$Dy and $163$Dy nucleus in anionic DyPc$.
arXiv Detail & Related papers (2020-02-12T18:25:31Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.