Electron-spin spectral diffusion in an erbium doped crystal at
millikelvin temperatures
- URL: http://arxiv.org/abs/2203.15012v1
- Date: Mon, 28 Mar 2022 18:20:47 GMT
- Title: Electron-spin spectral diffusion in an erbium doped crystal at
millikelvin temperatures
- Authors: Milos Ran\v{c}i\'c, Marianne Le Dantec, Sen Lin, Sylvain Bertaina,
Thierry Chaneli\`ere, Diana Serrano, Philippe Goldner, Ren Bao Liu, Emmanuel
Flurin, Daniel Est\`eve, Denis Vion and Patrice Bertet
- Abstract summary: We characterize the spectral diffusion processes that limit the electron-spin coherence of Er ions at millikelvin temperatures.
The coherence time shows a strong temperature dependence, reaching 1.3 ms at 23 mK for an electron-spin transition of $167textEr$.
- Score: 0.8961088845748072
- License: http://creativecommons.org/licenses/by-nc-nd/4.0/
- Abstract: Erbium-doped crystals offer a versatile platform for hybrid quantum devices
because they combine magnetically-sensitive electron-spin transitions with
telecom-wavelength optical transitions. At the high doping concentrations
necessary for many quantum applications, however, strong magnetic interactions
of the electron-spin bath lead to excess spectral diffusion and rapid
decoherence. Here we lithographically fabricate a 4.4 GHz superconducting
planar micro-resonator on a $\text{CaWO}_{4}$ crystal doped with Er ions at a
concentration of twenty parts per million relative to Ca. Using the microwave
resonator, we characterize the spectral diffusion processes that limit the
electron-spin coherence of Er ions at millikelvin temperatures by applying 2-
and 3-pulse echo sequences. The coherence time shows a strong temperature
dependence, reaching 1.3 ms at 23 mK for an electron-spin transition of
$^{167}\text{Er}$.
Related papers
- Electron Paramagnetic Resonance spectroscopy of a scheelite crystal
using microwave photon counting [0.0]
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has been introduced as a sensitive new method for electron paramagnetic resonance spectroscopy at millikelvin temperatures.
Here, we apply this spin fluorescence method to a scheelite crystal of CaWO4.
arXiv Detail & Related papers (2024-02-05T15:30:56Z) - Transition metal ion ensembles in crystals as solid-state coherent
spin-photon interfaces: The case of nickel in magnesium oxide [0.0]
We present general guidelines for finding solid-state systems that could serve as coherent electron spin-photon interfaces.
We show that transition metal ions in various crystals could comply with these guidelines.
arXiv Detail & Related papers (2022-12-30T17:10:04Z) - Coherent spin dynamics of rare-earth doped crystals in the
high-cooperativity regime [0.7586208381054043]
Rare-earth doped crystals have long coherence times and the potential to provide quantum interfaces between microwave and optical photons.
We measure spin dynamics of two rare-earth spin species, $145$Nd and Yb doped into Y$_2$SiO$_5$, coupled to a planar microwave resonator in the high cooperativity regime.
We identify relevant decoherence mechanisms including instantaneous diffusion arising from resonant spins and temperature-dependent spectral diffusion from impurity electron and nuclear spins.
arXiv Detail & Related papers (2022-06-08T17:36:59Z) - Near-monochromatic tuneable cryogenic niobium electron field emitter [48.7576911714538]
We describe electron field emission from a monocrystalline, superconducting niobium nanotip at a temperature of 5.9 K.
The emitted electron energy spectrum reveals an ultra-narrow distribution down to 16 meV.
This source will decrease the impact of lens aberration and enable new modes in low-energy electron microscopy, electron energy loss spectroscopy, and high-resolution vibrational spectroscopy.
arXiv Detail & Related papers (2022-05-11T20:46:21Z) - Single quantum emitters with spin ground states based on Cl bound
excitons in ZnSe [55.41644538483948]
We show a new type of single photon emitter with potential electron spin qubit based on Cl impurities inSe.
Results suggest single Cl impurities are suitable as single photon source with potential photonic interface.
arXiv Detail & Related papers (2022-03-11T04:29:21Z) - Twenty-three millisecond electron spin coherence of erbium ions in a
natural-abundance crystal [0.8331845551768636]
This is the longest electron spin coherence time measured in a material with a natural abundance of nuclear spins.
Our results establish Er$3+$:CaWO$_4$ as a leading platform for quantum networks.
arXiv Detail & Related papers (2021-06-28T20:45:11Z) - Algorithmic Ground-state Cooling of Weakly-Coupled Oscillators using
Quantum Logic [52.77024349608834]
We introduce a novel algorithmic cooling protocol for transferring phonons from poorly- to efficiently-cooled modes.
We demonstrate it experimentally by simultaneously bringing two motional modes of a Be$+$-Ar$13+$ mixed Coulomb crystal close to their zero-point energies.
We reach the lowest temperature reported for a highly charged ion, with a residual temperature of only $Tlesssim200mathrmmu K$ in each of the two modes.
arXiv Detail & Related papers (2021-02-24T17:46:15Z) - Broad-band spectroscopy of a vanadyl porphyrin: a model electronuclear
spin qudit [0.0]
We show that each molecule fulfills the conditions to act as a universal 4-qubit processor or, equivalently, as a d = 16 qudit.
These findings widen the catalogue of chemically designed systems able to implement non-trivial quantum functionalities.
arXiv Detail & Related papers (2021-01-27T19:12:23Z) - Photon Condensation and Enhanced Magnetism in Cavity QED [68.8204255655161]
A system of magnetic molecules coupled to microwave cavities undergoes the equilibrium superradiant phase transition.
The effect of the coupling is first illustrated by the vacuum-induced ferromagnetic order in a quantum Ising model.
A transmission experiment is shown to resolve the transition, measuring the quantum electrodynamical control of magnetism.
arXiv Detail & Related papers (2020-11-07T11:18:24Z) - Electrically tuned hyperfine spectrum in neutral
Tb(II)(Cp$^{\rm{iPr5}}$)$_2$ single-molecule magnet [64.10537606150362]
Both molecular electronic and nuclear spin levels can be used as qubits.
In solid state systems with dopants, an electric field was shown to effectively change the spacing between the nuclear spin qubit levels.
This hyperfine Stark effect may be useful for applications of molecular nuclear spins for quantum computing.
arXiv Detail & Related papers (2020-07-31T01:48:57Z) - Optimal coupling of HoW$_{10}$ molecular magnets to superconducting
circuits near spin clock transitions [85.83811987257297]
We study the coupling of pure and magnetically diluted crystals of HoW$_10$ magnetic clusters to microwave superconducting coplanar waveguides.
Results show that engineering spin-clock states of molecular systems offers a promising strategy to combine sizeable spin-photon interactions with a sufficient isolation from unwanted magnetic noise sources.
arXiv Detail & Related papers (2019-11-18T11:03:06Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.