Oxygen Vacancies in Niobium Pentoxide as a Source of Two-Level System Losses in Superconducting Niobium

• URL: http://arxiv.org/abs/2108.13352v3
• Date: Wed, 24 Apr 2024 21:03:06 GMT
• Title: Oxygen Vacancies in Niobium Pentoxide as a Source of Two-Level System Losses in Superconducting Niobium
• Authors: Daniel Bafia, Akshay Murthy, Anna Grassellino, Alexander Romanenko,
• Abstract summary: oxygen vacancies in the niobium pentoxide drive two-level system (TLS) losses. We identify a major source of quantum decoherence in three-dimensional superconducting radio-frequency (SRF) resonators and two-dimensional transmon qubits composed of oxidized niobium.
• Score: 41.94295877935867
• License: http://creativecommons.org/licenses/by/4.0/
• Abstract: We identify a major source of quantum decoherence in three-dimensional superconducting radio-frequency (SRF) resonators and two-dimensional transmon qubits composed of oxidized niobium: oxygen vacancies in the niobium pentoxide which drive two-level system (TLS) losses. By probing the effect of sequential \textit{in situ} vacuum baking treatments on the RF performance of bulk Nb SRF resonators and on the oxide structure of a representative Nb sample using time-of-flight secondary ion mass spectrometry (ToF-SIMS), we find a non-monotonic evolution of cavity quality factor $Q_0$ which correlates with the interplay of Nb\textsubscript{2}O\textsubscript{5} vacancy generation and oxide thickness reduction. We localize this effect to the oxide itself and present the insignificant role of diffused interstitial oxygen in the underlying Nb by regrowing a new oxide \textit{via} wet oxidation which reveals a mitigation of aggravated TLS losses. We hypothesize that such vacancies in the pentoxide serve as magnetic impurities and are a source of TLS-driven RF loss.

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