Exciton Dynamics and Time-Resolved Fluorescence in Nanocavity-Integrated Monolayers of Transition-Metal Dichalcogenides

• URL: http://arxiv.org/abs/2303.15470v1
• Date: Sat, 25 Mar 2023 10:13:43 GMT
• Title: Exciton Dynamics and Time-Resolved Fluorescence in Nanocavity-Integrated Monolayers of Transition-Metal Dichalcogenides
• Authors: Kewei Sun, Kaijun Shen, Maxim F. Gelin and Yang Zhao
• Abstract summary: We have developed an ab-initio-based numerically-accurate methodology for the simulation of the exciton dynamics and time- and frequency-resolved fluorescence spectra of the cavity-controlled materials at finite temperature. This allowed us to establish dynamical and spectroscopic signatures of the polaronic and polaritonic effects as well as uncover their characteristic timescales in the relevant range of temperatures.
• Score: 9.960057330841405
• License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
• Abstract: We have developed an ab-initio-based fully-quantum numerically-accurate methodology for the simulation of the exciton dynamics and time- and frequency-resolved fluorescence spectra of the cavity-controlled two-dimensional materials at finite temperature and applied this methodology to the single-layer WSe2 system. This allowed us to establish dynamical and spectroscopic signatures of the polaronic and polaritonic effects as well as uncover their characteristic timescales in the relevant range of temperatures.

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