Two-dimensional shelving spectroscopy of ultraviolet ground state transitions in dysprosium
- URL: http://arxiv.org/abs/2604.07283v1
- Date: Wed, 08 Apr 2026 16:44:52 GMT
- Title: Two-dimensional shelving spectroscopy of ultraviolet ground state transitions in dysprosium
- Abstract summary: Here, we investigate multiple ultraviolet (UV) ground state transitions in dysprosium.<n>Several of these UV excited states have the largest decay strengths to the ultralong-lived, low-lying first excited state.<n>We measure isotope shifts, hyperfine coefficients, and create King plots to determine their electronic nature.
- Score: 0.0
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: The open inner-shell electronic structure of lanthanides with large magnetic moments gives rise to a rich spectrum of transitions available for laser cooling, trapping, and coherent control. Despite this, the large number of ultraviolet (UV) transitions below 400nm have so far been rarely utilized in dipolar atom experiments. Here, we investigate multiple UV ground state transitions in dysprosium. Several of these UV excited states have the largest decay strengths to the ultralong-lived, low-lying first excited state which are comparable to the most commonly used strongest transitions found in dipolar atoms. Using two-dimensional shelving spectroscopy which improves detection sensitivity and provides a straightforward way to determine the hyperfine-isotope structure and excited state total angular momentum $J$, we measure isotope shifts, hyperfine coefficients, and create King plots to determine their electronic nature. Such knowledge of these UV transitions which analogously exist in other magnetic atoms is important for optically populating the first excited state and can be used towards creating an optical clock, high resolution imaging in quantum gas microscopy, and probing lanthanide nuclei with enhanced Schiff moments in search of physics beyond the standard model.
Related papers
- Optically Resolved Excited State Hyperfine Structure of a Silicon Colour Centre in the Telecom Bands [0.0]
Nuclear spinbits in silicon offer exceptionally coherent quantum memory.<n>Optical-interfaced spins are a promising platform for both quantum networking and distributed quantum computing.<n>We measure the excited-state lifetimes and, as a consequence of its narrow emission linewidth, observe the fine and hyperfine structure of the long-lived triplet state.
arXiv Detail & Related papers (2026-07-31T01:54:04Z) - Experimental Verification of Electron-Photon Entanglement [39.58317527488534]
Entanglement, a key resource of emerging quantum technologies, describes correlations between particles that defy classical physics.<n>We demonstrate entanglement in electron-photon pairs generated via cathodoluminescence in a transmission electron microscope.<n>Our work paves the way for exploring quantum correlations in free-electron systems and their application to quantum-enhanced imaging techniques on the nanoscale.
arXiv Detail & Related papers (2025-04-17T17:58:50Z) - The role of spectator modes in the quantum-logic spectroscopy of single trapped molecular ions [39.146761527401424]
Quantum-logic spectroscopy has become an increasingly important tool for the state detection and readout of trapped atomic and molecular ions.<n>In this approach, the internal state of the target ion is mapped onto a co-trapped auxiliary ion.<n>The present study investigates the role of spectator modes not directly involved in a measurement protocol relying on a state-dependent optical-dipole force.
arXiv Detail & Related papers (2025-04-03T14:37:24Z) - Photon bunching in high-harmonic emission controlled by quantum light [0.0]
Recent theories have laid the groundwork for understanding how quantum-optical properties affect high-field photonics.
We demonstrate a new experimental approach that transduces some properties of a quantum-optical state through a strong-field nonlinearity.
Our results suggest that perturbing strong-field dynamics with quantum-optical states is a viable way to coherently control the generation of these states at short wavelengths.
arXiv Detail & Related papers (2024-04-08T12:53:42Z) - Room-temperature quantum sensing with photoexcited triplet electrons in organic crystals [1.4085555227308877]
Quantum sensors constructed from polarized spintriplet electrons in photoexcited organic chromophores.<n>Technology highlights new potential for quantum sensing in chemical systems.
arXiv Detail & Related papers (2024-02-21T16:09:49Z) - In-situ-tunable spin-spin interactions in a Penning trap with in-bore
optomechanics [41.94295877935867]
We present an optomechanical system for in-situ tuning of the coherent spin-motion and spin-spin interaction strength.
We characterize the system using measurements of the induced mean-field spin precession.
These experiments show approximately a $times2$ variation in the ratio of the coherent to incoherent interaction strength.
arXiv Detail & Related papers (2024-01-31T11:00:39Z) - Engineering quantum control with twisted-light fields induced optical
transitions [0.0]
A novel form of quantum control is proposed by applying twisted-light also known as optical vortex beams.
This method introduces spatially tailored electric and magnetic fields to rewrite atomic selection rules.
Engineering light-matter interaction by optical vortices will benefit to experimental atomic and molecular platforms.
arXiv Detail & Related papers (2023-06-30T12:51:23Z) - Observation of superradiant bursts in a cascaded quantum system [0.0]
Dicke superradiance describes the collective radiative decay of a fully inverted ensemble of two-level atoms.
We experimentally investigate this effect for a chiral, i.e.,direction-dependent light--matter coupling.
Our results shed light on the collective radiative dynamics of cascaded quantum many-body systems.
arXiv Detail & Related papers (2022-11-16T14:36:10Z) - Universal pair-polaritons in a strongly interacting Fermi gas [0.0]
We report on experiments using molecular transitions in a strongly interacting Fermi gas, directly coupling cavity photons to pairs of atoms.
The dependence of the pair-polariton spectrum on interatomic interactions is universal, independent of the transition used.
This represents a magnification of many-body effects by two orders of magnitude in energy.
arXiv Detail & Related papers (2021-03-03T15:06:06Z) - Position-controlled quantum emitters with reproducible emission
wavelength in hexagonal boron nitride [45.39825093917047]
Single photon emitters (SPEs) in low-dimensional layered materials have recently gained a large interest owing to the auspicious perspectives of integration and extreme miniaturization.
Here, we evidence SPEs in high purity synthetic hexagonal boron nitride (hBN) that can be activated by an electron beam at chosen locations.
Our findings constitute an essential step towards the realization of top-down integrated devices based on identical quantum emitters in 2D materials.
arXiv Detail & Related papers (2020-11-24T17:20:19Z) - Spectrally reconfigurable quantum emitters enabled by optimized fast
modulation [42.39394379814941]
Spectral control in solid state platforms such as color centers, rare earth ions, and quantum dots is attractive for realizing such applications on-chip.
We propose the use of frequency-modulated optical transitions for spectral engineering of single photon emission.
Our results suggest that frequency modulation is a powerful technique for the generation of new light states with unprecedented control over the spectral and temporal properties of single photons.
arXiv Detail & Related papers (2020-03-27T18:24:35Z) - Optical projection and spatial separation of spin entangled
triplet-pairs from the S1 (21Ag-) state of pi-conjugated systems [40.96261204117952]
We experimentally demonstrate that S1 (21Ag-) is a superposition state with strong contributions from spin-entangled pairs of triplet excitons (1(TT))
We show that optical manipulation of the S1 (21Ag-) wavefunction using triplet absorption transitions allows selective projection of the 1(TT) component into a manifold of spatially separated triplet-pairs with lifetimes enhanced by up to one order of magnitude.
Our results provide a unified picture of 21Ag-states in pi-conjugated materials and open new routes to exploit their dynamics in singlet fission, photobiology and for the
arXiv Detail & Related papers (2020-02-27T22:09:43Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.