Entangled biphoton enhanced double quantum coherence signal as a probe for cavity polariton correlations in presence of phonon induced dephasing

• URL: http://arxiv.org/abs/2205.15698v2
• Date: Sun, 26 Jun 2022 10:53:07 GMT
• Title: Entangled biphoton enhanced double quantum coherence signal as a probe for cavity polariton correlations in presence of phonon induced dephasing
• Authors: Arunangshu Debnath and Angel Rubio
• Abstract summary: We propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phonon-induced dissipation.
• Score: 0.0
• License: http://creativecommons.org/licenses/by/4.0/
• Abstract: We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phonon-induced dissipation. The non-classicality of the entangled biphoton sources is shown to enhance the ultra-fast and broadband correlation features of the signal, giving an indication about the underlying state correlations responsible for long-range cavity-assisted exciton migration.

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