Homogeneous electron gas in arbitrary dimensions beyond the random phase approximation

• URL: http://arxiv.org/abs/2210.03024v2
• Date: Fri, 7 Oct 2022 06:15:47 GMT
• Title: Homogeneous electron gas in arbitrary dimensions beyond the random phase approximation
• Authors: L. V. Duc Pham, Pascal Sattler, Miguel A. L. Marques, and Carlos L. Benavides-Riveros
• Abstract summary: We use the celebrated approach developed by Singwi, Tosi, Land, and Sj"olander (STLS) to compute correlation energy beyond the random phase approximation (RPA) For two and three dimensions, both in the paramagnetic and ferromagnetic ground states, STLS is capable of producing correlation energies in close agreement with Monte-Carlo values.
• Score: 0.0
• License: http://creativecommons.org/licenses/by/4.0/
• Abstract: The ground state of the homogeneous electron gas is a cornerstone in quantum physics and chemistry. It is an archetypal system in the regime of slowly varying densities in which the exchange-correlation energy can be estimated with a myriad of methods. For high densities, the behavior of the energy is well-known for 1, 2, and 3 dimensions. Here, we extend this model to arbitrary integer dimensions, and compute its correlation energy beyond the random phase approximation (RPA), using the celebrated approach developed by Singwi, Tosi, Land, and Sj\"olander (STLS), which is known to be remarkably accurate in the description of the full electronic density response. For two and three dimensions, both in the paramagnetic and ferromagnetic ground states, STLS is capable of producing correlation energies in close agreement with Monte-Carlo values. For higher dimensions, we compare the results obtained for the correlation energy using the STLS method with the values previously obtained using RPA. We furthermore illustrate the importance of the plasmon contribution to STLS theory.

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