Zero field magnetic resonance spectroscopy based on Nitrogen-vacancy
centers
- URL: http://arxiv.org/abs/2304.02179v1
- Date: Wed, 5 Apr 2023 01:08:54 GMT
- Title: Zero field magnetic resonance spectroscopy based on Nitrogen-vacancy
centers
- Authors: Linkai Zhao, Q. Chen
- Abstract summary: We propose a scheme to have zero field magnetic resonance spectroscopy based on a nitrogen-vacancy center.
Our work extends applications of NV centers as a nanoscale molecule spectroscopy in the zero field regime.
- Score: 0.0
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: We propose a scheme to have zero field magnetic resonance spectroscopy based
on a nitrogen-vacancy center and investigate the new applications in which
magnetic bias field might disturb the system under investigation. Continual
driving with circularly polarized microwave fields is used to selectively
address one spin state. The proposed method is applied for single molecule
spectroscopy, such as nuclear quadrupole resonance spectroscopy of a $^{11}$B
nuclear spin and the detection of the distance of two hydrogen nuclei in a
water molecule. Our work extends applications of NV centers as a nanoscale
molecule spectroscopy in the zero field regime.
Related papers
- Quantum control of ro-vibrational dynamics and application to
light-induced molecular chirality [39.58317527488534]
Achiral molecules can be made temporarily chiral by excitation with electric fields.
We go beyond the assumption of molecular orientations to remain fixed during the excitation process.
arXiv Detail & Related papers (2023-10-17T20:33:25Z) - In situ electron paramagnetic resonance spectroscopy using single
nanodiamond sensors [11.37424763147048]
We show a zero-field EPR technique with spectra robust to the sensor's orientation.
We acquire the zero-field EPR spectrum of vanadyl ions in glycerol solution with embedded single NDs.
arXiv Detail & Related papers (2023-07-25T09:07:56Z) - Sensing of magnetic field effects in radical-pair reactions using a
quantum sensor [50.591267188664666]
Magnetic field effects (MFE) in certain chemical reactions have been well established in the last five decades.
We employ elaborate and realistic models of radical-pairs, considering its coupling to the local spin environment and the sensor.
For two model systems, we derive signals of MFE detectable even in the weak coupling regime between radical-pair and NV quantum sensor.
arXiv Detail & Related papers (2022-09-28T12:56:15Z) - High-resolution spectroscopy of a single nitrogen-vacancy defect at zero
magnetic field [0.3848364262836075]
We report a study of high-resolution microwave spectroscopy of nitrogen-vacancy centers in diamond crystals at and around zero magnetic field.
We observe characteristic splitting and transition imbalance of the hyperfine transitions, which originate from level anti-crossings in the presence of a transverse effective field.
Our results are of importance for the optimization of the experimental conditions for the polarization-selective microwave excitation of spin-1 systems in zero or weak magnetic fields.
arXiv Detail & Related papers (2022-06-30T02:49:49Z) - Quantum Heterodyne Sensing of Nuclear Spins via Double Resonance [0.0]
A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral resolution.
This work paves the way towards high field nanoscale heterodyne NMR protocols with NV centres.
arXiv Detail & Related papers (2022-05-20T13:48:59Z) - Multi-Center Magnon Excitations Open the Entire Brillouin Zone to
Terahertz Magnetometry of Quantum Magnets [42.72559625804617]
The magnon density of states can be accessed over the entire Brillouin zone through three-center magnon excitations.
The results of THz time-domain experiments agree remarkably well with linear spin-wave theory.
arXiv Detail & Related papers (2022-03-08T19:04:24Z) - Dispersive readout of molecular spin qudits [68.8204255655161]
We study the physics of a magnetic molecule described by a "giant" spin with multiple $d > 2$ spin states.
We derive an expression for the output modes in the dispersive regime of operation.
We find that the measurement of the cavity transmission allows to uniquely determine the spin state of the qudits.
arXiv Detail & Related papers (2021-09-29T18:00:09Z) - Controlled coherent dynamics of [VO(TPP)], a prototype molecular nuclear
qudit with an electronic ancilla [50.002949299918136]
We show that [VO(TPP)] (vanadyl tetraphenylporphyrinate) is a promising system suitable to implement quantum computation algorithms.
It embeds an electronic spin 1/2 coupled through hyperfine interaction to a nuclear spin 7/2, both characterized by remarkable coherence.
arXiv Detail & Related papers (2021-03-15T21:38:41Z) - Cross-relaxation studies with optically detected magnetic resonances in
nitrogen-vacancy centers in diamond in an external magnetic field [0.0]
Cross-relaxation between nitrogen-vacancy centers and substitutional nitrogen in a diamond crystal was studied.
Optically detected magnetic resonance signals (ODMR) can be used to measure these signals successfully.
arXiv Detail & Related papers (2020-07-01T13:23:22Z) - Kilohertz electron paramagnetic resonance spectroscopy of single
nitrogen centers at zero magnetic field [9.976365365803575]
nitrogen-vacancy centers in diamond serve as an atomic-sized magnetometer.
Current megahertz spectral resolution is still insufficient to resolve key heterogeneous molecular information.
We demonstrate a 27-fold narrower spectrum of single substitutional nitrogen centers in diamond with linewidth of several kilohertz.
arXiv Detail & Related papers (2020-05-29T17:59:48Z) - Two-Dimensional Single- and Multiple-Quantum Correlation Spectroscopy in
Zero-Field Nuclear Magnetic Resonance [55.41644538483948]
We present single- and multiple-quantum correlation $J$-spectroscopy detected in zero magnetic field using a Rb vapor-cell magnetometer.
At zero field the spectrum of ethanol appears as a mixture of carbon isotopomers, and correlation spectroscopy is useful in separating the two composite spectra.
arXiv Detail & Related papers (2020-04-09T10:02:45Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.