Reconstructing the spatial structure of quantum correlations in materials
- URL: http://arxiv.org/abs/2306.11723v3
- Date: Tue, 27 Aug 2024 21:52:32 GMT
- Title: Reconstructing the spatial structure of quantum correlations in materials
- Authors: Allen Scheie, Pontus Laurell, Elbio Dagotto, D. Alan Tennant, Tommaso Roscilde,
- Abstract summary: Quantum correlations are a fundamental property of many-body states.
Yet they remain elusive, hindering certification of genuine quantum materials.
We show that momentumdependent dynamical behavior via neutron scattering enables a general family of quantum correlation.
- Score: 0.0
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: Quantum correlations are a fundamental property of quantum many-body states. Yet they remain experimentally elusive, hindering certification of genuine quantum behavior, especially in quantum materials. Here we show that the momentum-dependent dynamical susceptibility measured via inelastic neutron scattering enables the systematic reconstruction of a general family of quantum correlation functions, which express the degree of quantum coherence in the fluctuations of two spins at arbitrary mutual distance. Using neutron scattering data on the compound KCuF$_3$ $\unicode{x2014}$ a system of weakly coupled $S=1/2$ Heisenberg chains $\unicode{x2014}$ and of numerically exact quantum Monte Carlo data, we show that quantum correlations possess a radically different spatial structure with respect to conventional correlations. Indeed, they exhibit a new emergent length scale $\unicode{x2014}$ the quantum coherence length $\unicode{x2014}$ which is finite at any finite temperature (including when long-range magnetic order develops). Moreover, we show theoretically that coupled Heisenberg spin chains exhibit a form of quantum monogamy, with a trade-off between quantum correlations along and transverse to the spin chains. These results highlight real-space quantum correlators as an informative, model-independent means of probing the underlying quantum state of real quantum materials.
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