Enhanced coherent light-matter interaction and room-temperature quantum
yield of plasmonic resonances engineered by a chiral exceptional point
- URL: http://arxiv.org/abs/2308.04239v1
- Date: Tue, 8 Aug 2023 13:10:04 GMT
- Title: Enhanced coherent light-matter interaction and room-temperature quantum
yield of plasmonic resonances engineered by a chiral exceptional point
- Authors: Yuwei Lu, Haoxiang Jiang, Renming Liu
- Abstract summary: We propose to tailor the local density of states (LDOS) of plasmonic resonances by integrating with a photonic cavity operating at a chiral exceptional point (CEP)
A quantized few-mode theory is employed to reveal that the LDOS of the proposed hybrid cavity can evolve into sub-tzian lineshape, with order-of-magnitude linewidth narrowing.
This results in the enhanced coherent light-matter interaction accompanied by the reduced dissipation of polaritonic states.
- Score: 1.074267520911262
- License: http://creativecommons.org/licenses/by/4.0/
- Abstract: Strong dissipation of plasmonic resonances is detrimental to quantum
manipulation. To enhance the quantum coherence, we propose to tailor the local
density of states (LDOS) of plasmonic resonances by integrating with a photonic
cavity operating at a chiral exceptional point (CEP), where the phase of light
field can offer a new degree of freedom to flexibly manipulate the quantum
states. A quantized few-mode theory is employed to reveal that the LDOS of the
proposed hybrid cavity can evolve into sub-Lorentzian lineshape, with
order-of-magnitude linewidth narrowing and additionally a maximum of eightfold
enhancement compared to the usual plasmonic-photonic cavity without CEP. This
results in the enhanced coherent light-matter interaction accompanied by the
reduced dissipation of polaritonic states. Furthermore, a scattering theory
based on eigenmode decomposition is present to elucidate two mechanisms
responsible for the significant improvement of quantum yield at CEP, the
reduction of plasmonic absorption by the Fano interference and the enhancement
of cavity radiation through the superscattering. Importantly, we find the
latter allows achieving a near-unity quantum yield at room temperature; in
return, high quantum yield is beneficial to experimentally verify the enhanced
LDOS at CEP by measuring the fluorescence lifetime of a quantum emitter.
Therefore, our work demonstrates that the plasmonic resonances in
CEP-engineered environment can serve as a promising platform for exploring the
quantum states control by virtue of the non-Hermiticity of open optical
resonators and building the high-performance quantum devices for sensing,
spectroscopy, quantum information processing and quantum computing.
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