High-purity and stable single-photon emission in bilayer WSe$_2$ via phonon-assisted excitation

• URL: http://arxiv.org/abs/2406.07097v1
• Date: Tue, 11 Jun 2024 09:37:59 GMT
• Title: High-purity and stable single-photon emission in bilayer WSe$_2$ via phonon-assisted excitation
• Authors: Claudia Piccinini, Athanasios Paralikis, José Ferreira Neto, Abdulmalik Abdulkadir Madigawa, Paweł Wyborski, Vikas Remesh, Luca Vannucci, Niels Gregersen, Battulga Munkhbat,
• Abstract summary: We investigate the impact of different optical excitation strategies on the single-photon emission characteristics of bilayer WSe$$$ quantum emitters. Under phonon-assisted excitation, we achieve narrow and stable single-photon emission with an excellent purity reaching $ 0.94pm 0.02,$.
• Score: 0.0
• License: http://creativecommons.org/licenses/by/4.0/
• Abstract: The excitation scheme is essential for single-photon sources as it prepares the exciton state, defines the decay dynamics, and influences the spectral diffusion of the emitted single photons. Here, we investigate the impact of different optical excitation strategies on the single-photon emission characteristics of bilayer WSe$_2$ quantum emitters. Under phonon-assisted excitation, we achieve narrow and stable single-photon emission with an excellent purity reaching $ 0.94\pm 0.02\,$. Furthermore, the decay time is reduced by more than an order of magnitude from $(16.65 \pm 2.39)\,$ns for above-band excitation to $(1.33 \pm 0.04)\,$ns for phonon-assisted excitation. Finally, we observe a suppressed spectral wandering along with a two-fold reduction of the spectral linewidth. Our comprehensive investigation highlights the critical role of the excitation method in optimizing the performance of WSe$_2$-based quantum emitters.

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