Spectral function of a bipolaron coupled to dispersive optical phonons

• URL: http://arxiv.org/abs/2410.11537v2
• Date: Wed, 15 Jan 2025 10:52:16 GMT
• Title: Spectral function of a bipolaron coupled to dispersive optical phonons
• Authors: K. Kovač, J. Bonča,
• Abstract summary: We study the interplay between phonon dispersion and Coulomb repulsion and their effects on the single-electron removal spectral function. The spectral function is significantly influenced by phonon dispersion, particularly in systems with strong electron-phonon coupling.
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• Abstract: Using an efficient variational exact diagonalization method, we computed the electron removal spectral function within the framework of the Holstein-Hubbard model containing two electrons with opposite spins coupled to dispersive quantum optical phonons. Our primary focus was examining the interplay between phonon dispersion and Coulomb repulsion and their effects on the single-electron removal spectral function, relevant for the analysis of angle-resolved photoemission spectroscopy (ARPES). Tuning the strengths of the electron-phonon coupling and the Hubbard interaction allows us to examine the evolution of the spectral properties of the system as it crosses over from a bound bipolaron to separate polarons. With increasing Hubbard repulsion, the decrease of the bipolaron binding energy results in the gradual downward shift of the polaron band - a low-frequency feature in the spectral function. Simultaneously, the intensity of the polaron band away from the center of the Brillouin zone diminishes until it remains non-zero only in its center as the bipolaron unbinds into two separate polarons. The spectral function is significantly influenced by phonon dispersion, particularly in systems with strong electron-phonon coupling. The sign of the curvature of the phonon band plays a crucial role in the distribution of spectral weight.

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