Observation of non-adiabatic Landau-Zener tunneling among Floquet states
- URL: http://arxiv.org/abs/2503.04431v1
- Date: Thu, 06 Mar 2025 13:44:21 GMT
- Title: Observation of non-adiabatic Landau-Zener tunneling among Floquet states
- Authors: Yun Yen, Marcel Reutzel, Andi Li, Zehua Wang, Hrvoje Petek, Michael Schüler,
- Abstract summary: Floquet engineering provides a powerful framework to dress electronic states with time-periodic fields.<n>Non-perturbative responses of the dressed states emerge, yet their nonlinear dynamics remain challenging to interpret.<n>Our results establish a direct connection the onset of light-dressing of matter, non-perturbative ultrafast lightwave electronics, and high-optical-harmonic generation in the solids.
- Score: 1.9243512902867335
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: Electromagnetic fields not only induce electronic transitions but also fundamentally modify the quantum states of matter through strong light-matter interactions. As one established route, Floquet engineering provides a powerful framework to dress electronic states with time-periodic fields, giving rise to quasi-stationary Floquet states. With increasing field strength, non-perturbative responses of the dressed states emerge, yet their nonlinear dynamics remain challenging to interpret. In this work we explore the emergence of non-adiabatic Landau-Zener transitions among Floquet states in Cu(111) under intense optical fields. At increasing field strength, we observe a transition from perturbative dressing to a regime where Floquet states undergo non-adiabatic tunneling, revealing a breakdown of adiabatic Floquet evolution. These insights are obtained through interferometrically time-resolved multi-photon photoemission spectroscopy, which serves as a sensitive probe of transient Floquet state dynamics. Numerical simulations and the theory of instantaneous Floquet states allow us to directly examine real-time excitation pathways in this non-perturbative photoemission regime. Our results establish a direct connection the onset of light-dressing of matter, non-perturbative ultrafast lightwave electronics, and high-optical-harmonic generation in the solids.
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