PINEAPPLE: Physics-Informed Neuro-Evolution Algorithm for Prognostic Parameter Inference in Lithium-Ion Battery Electrodes
- URL: http://arxiv.org/abs/2602.18042v1
- Date: Fri, 20 Feb 2026 07:51:59 GMT
- Title: PINEAPPLE: Physics-Informed Neuro-Evolution Algorithm for Prognostic Parameter Inference in Lithium-Ion Battery Electrodes
- Authors: Karkulali Pugalenthi, Jian Cheng Wong, Qizheng Yang, Pao-Hsiung Chiu, My Ha Dao, Nagarajan Raghavan, Chinchun Ooi,
- Abstract summary: PINEAPPLE is a novel framework that integrates physics-informed neural networks (PINNs) with an evolutionary search algorithm to enable rapid, scalable, and interpretable parameter inference.<n> PINEAPPLE demonstrates robust parameter inference solely from voltage-time discharge curves across multiple batteries from the open-source CALCE repository.<n>By enabling computationally efficient, real-time parameter estimation, PINEAPPLE offers a promising route towards the non-destructive, physics-based characterization of inter-cell and intra-cell variability.
- Score: 0.8376229126363229
- License: http://creativecommons.org/licenses/by/4.0/
- Abstract: Accurate, real-time, yet non-destructive estimation of internal states in lithium-ion batteries is critical for predicting degradation, optimizing usage strategies, and extending operational lifespan. Here, we introduce PINEAPPLE (Physics-Informed Neuro-Evolution Algorithm for Prognostic Parameter inference in Lithium-ion battery Electrodes), a novel framework that integrates physics-informed neural networks (PINNs) with an evolutionary search algorithm to enable rapid, scalable, and interpretable parameter inference with potential for application to next-generation batteries. The meta-learned PINN utilizes fundamental physics principles to achieve accurate zero-shot prediction of electrode behavior with test errors below 0.1$\%$ while maintaining an order-of-magnitude speed-up over conventional solvers. PINEAPPLE demonstrates robust parameter inference solely from voltage-time discharge curves across multiple batteries from the open-source CALCE repository, recovering the evolution of key internal state parameters such as Li-ion diffusion coefficients across usage cycles. Notably, the inferred cycle-dependent evolution of these parameters exhibit consistent trends across different batteries without any customized degradation physics-embedded heuristic, highlighting the effective regularizing effect and robustness that can be conferred through incorporation of fundamental physics in PINEAPPLE. By enabling computationally efficient, real-time parameter estimation, PINEAPPLE offers a promising route towards the non-destructive, physics-based characterization of inter-cell and intra-cell variability of battery modules and battery packs, thereby unlocking new opportunities for downstream on-the-fly needs in next-generation battery management systems such as individual cell-scale state-of-health diagnostics.
Related papers
- EntroLnn: Entropy-Guided Liquid Neural Networks for Operando Refinement of Battery Capacity Fade Trajectories [5.440491961792461]
This study extends the scope to online refinement of the entire capacity fade trajectory (CFT) through EntroLnn.<n>We introduce entropy-based features derived from online temperature fields, applied for the first time in battery analytics.<n>We achieve mean absolute errors of only 0.004577 for CFT and 18 cycles for EoL prediction.
arXiv Detail & Related papers (2026-01-08T03:32:57Z) - Fixed Point Neural Acceleration and Inverse Surrogate Model for Battery Parameter Identification [5.094264803596951]
We propose a deep learning-based framework for parameter identification of electrochemical battery models.<n>The proposed framework combines a neural surrogate model of the single particle model with electrolyte (NeuralSPMe) and a deep learning-based fixed-point iteration method.
arXiv Detail & Related papers (2025-10-28T07:20:38Z) - Modeling Membrane Degradation in PEM Electrolyzers with Physics-Informed Neural Networks [45.32169712547367]
Proton exchange membrane (PEM) electrolyzers are pivotal for sustainable hydrogen production.<n>Their long-term performance is hindered by membrane degradation, which poses reliability and safety challenges.<n>Traditional physics-based models have been developed, offering interpretability but requiring numerous parameters that are often difficult to measure and calibrate.<n>This study presents the first application of Physics-Informed Neural Networks (PINNs) to model membrane degradation in PEM electrolyzers.
arXiv Detail & Related papers (2025-06-19T15:46:49Z) - Accurate Ab-initio Neural-network Solutions to Large-Scale Electronic Structure Problems [52.19558333652367]
We present finite-range embeddings (FiRE) for accurate large-scale ab-initio electronic structure calculations.<n>FiRE reduces the complexity of neural-network variational Monte Carlo (NN-VMC) by $sim ntextel$, the number of electrons.<n>We validate our method's accuracy on various challenging systems, including biochemical compounds and organometallic compounds.
arXiv Detail & Related papers (2025-04-08T14:28:54Z) - On-site estimation of battery electrochemical parameters via transfer learning based physics-informed neural network approach [0.0]
The proposed approach significantly reduces computational costs, making it suitable for real-time implementation on battery management systems.<n>We have been able to effectively estimate relevant electrochemical parameters with operating data.<n>The methodology is experimentally validated in a Raspberry Pi device using data from a standard charge profile.
arXiv Detail & Related papers (2025-03-28T13:06:41Z) - Predicting ionic conductivity in solids from the machine-learned potential energy landscape [68.25662704255433]
We propose an approach for the quick and reliable screening of ionic conductors through the analysis of a universal interatomic potential.<n>Eight out of the ten highest-ranked materials are confirmed to be superionic at room temperature in first-principles calculations.<n>Our method achieves a speed-up factor of approximately 50 compared to molecular dynamics driven by a machine-learning potential, and is at least 3,000 times faster compared to first-principles molecular dynamics.
arXiv Detail & Related papers (2024-11-11T09:01:36Z) - PINN surrogate of Li-ion battery models for parameter inference. Part I: Implementation and multi-fidelity hierarchies for the single-particle model [0.0]
This manuscript is the first of a two-part series that introduces PINN surrogates of Li-ion battery models for parameter inference.
A multi-fidelity hierarchical training, where several neural nets are trained with multiple physics-loss fidelities is shown to significantly improve the surrogate accuracy.
arXiv Detail & Related papers (2023-12-28T19:09:56Z) - Enhanced physics-constrained deep neural networks for modeling vanadium
redox flow battery [62.997667081978825]
We propose an enhanced version of the physics-constrained deep neural network (PCDNN) approach to provide high-accuracy voltage predictions.
The ePCDNN can accurately capture the voltage response throughout the charge--discharge cycle, including the tail region of the voltage discharge curve.
arXiv Detail & Related papers (2022-03-03T19:56:24Z) - Physics-constrained deep neural network method for estimating parameters
in a redox flow battery [68.8204255655161]
We present a physics-constrained deep neural network (PCDNN) method for parameter estimation in the zero-dimensional (0D) model of the vanadium flow battery (VRFB)
We show that the PCDNN method can estimate model parameters for a range of operating conditions and improve the 0D model prediction of voltage.
We also demonstrate that the PCDNN approach has an improved generalization ability for estimating parameter values for operating conditions not used in the training.
arXiv Detail & Related papers (2021-06-21T23:42:58Z) - Modified Gaussian Process Regression Models for Cyclic Capacity
Prediction of Lithium-ion Batteries [5.663192900261267]
This paper presents the development of machine learning-enabled data-driven models for capacity predictions for lithium-ion batteries.
The developed models are validated compared on the Nickel Manganese Oxide (MCN) lithium-ion batteries with various cycling patterns.
arXiv Detail & Related papers (2020-12-31T19:05:27Z) - Benchmarking adaptive variational quantum eigensolvers [63.277656713454284]
We benchmark the accuracy of VQE and ADAPT-VQE to calculate the electronic ground states and potential energy curves.
We find both methods provide good estimates of the energy and ground state.
gradient-based optimization is more economical and delivers superior performance than analogous simulations carried out with gradient-frees.
arXiv Detail & Related papers (2020-11-02T19:52:04Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.