Measuring Time-Dependent Induced Quantum Coherences via Two-Dimensional
Coherence Spectroscopy
- URL: http://arxiv.org/abs/2104.03041v2
- Date: Tue, 23 Nov 2021 13:45:27 GMT
- Title: Measuring Time-Dependent Induced Quantum Coherences via Two-Dimensional
Coherence Spectroscopy
- Authors: William Barford, Allison Nicole Arber, Fynn McLennan, Max Marcus
- Abstract summary: We propose a two-dimensional spectroscopic protocol for measuring the time-dependent coherences between the stationary states of a system.
We also investigate the role of temporally-correlated noise on coherence dephasing.
- Score: 0.0
- License: http://creativecommons.org/licenses/by/4.0/
- Abstract: We propose a two-dimensional spectroscopic protocol for measuring the
time-dependent coherences between the stationary states of a system induced by
a time-dependent system-bath interaction. We also investigate the role of
temporally-correlated noise on coherence dephasing. This protocol enables
dynamical information about the system and its coupling to the environment to
be determined. Our results are based on the quantum-trajectory method, and are
obtained from both approximate, analytical and exact, numerical solutions of
the time-dependent Schroedinger equation. As an example, we show how this
protocol can be used to investigate exciton dynameds in conjugated polymers
induced by the coupling of their torsional modes with the environment.
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