Correlated driving-and-dissipation equation for non-Condon spectroscopy with the Herzberg-Teller vibronic coupling

• URL: http://arxiv.org/abs/2205.06413v1
• Date: Fri, 13 May 2022 01:37:16 GMT
• Title: Correlated driving-and-dissipation equation for non-Condon spectroscopy with the Herzberg-Teller vibronic coupling
• Abstract summary: Correlated driving-and-dissipation equation (CODDE) is an optimized complete second-order quantum dissipation approach. One can actually extract the hybridized bath dynamics from CODDE with the aid of dissipaton-equation-of-motion theory.
• Score: 8.152979330368892
• License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
• Abstract: Correlated driving-and-dissipation equation (CODDE) is an optimized complete second-order quantum dissipation approach, which is originally concerned with the reduced system dynamics only. However, one can actually extract the hybridized bath dynamics from CODDE with the aid of dissipaton-equation-of-motion theory, a statistical quasi-particle quantum dissipation formalism. Treated as an one{dissipaton theory, CODDE is successfully extended to deal with the Herzberg-Teller vibronic couplings in dipole-field interactions. Demonstrations will be carried out on the non-Condon spectroscopies of a model dimer system.

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