Entangled two-photon absorption in transmission-based experiments:
deleterious effects from linear optical losses
- URL: http://arxiv.org/abs/2310.07810v1
- Date: Wed, 11 Oct 2023 18:44:43 GMT
- Title: Entangled two-photon absorption in transmission-based experiments:
deleterious effects from linear optical losses
- Authors: Freiman Triana-Arango, Roberto Ram\'irez-Alarc\'on and Gabriel
Ramos-Ortiz
- Abstract summary: We present a new approach that exploits the properties of a Hong-Ou-Mandel (HOM) interferogram as a sensing device.
Here we analyze solutions of Rhodamine B (RhB), commonly used as a model of nonlinear medium in ETPA studies.
A detailed study of the effects of optical losses, unrelated to ETPA, over the HOM interferogram is carried out.
- Score: 0.0
- License: http://creativecommons.org/licenses/by/4.0/
- Abstract: Recently different experimental schemes have been proposed to study the
elusive phenomenon of entangled two-photon absorption (ETPA) in nonlinear
materials. The attempts to detect ETPA using transmission-based schemes have
led to results whose validity is currently under debate since the ETPA signal
can be corrupted or emulated by artifacts associated with linear optical
losses. The present work addresses the issue of linear losses and the
corresponding artifacts in transmission-based ETPA experiments through a new
approach that exploits the properties of a Hong-Ou-Mandel (HOM) interferogram.
Here we analyze solutions of Rhodamine B (RhB), commonly used as a model of
nonlinear medium in ETPA studies. Then, by using the HOM interferometer as a
sensing device, we firstly demonstrate the equivalence of the standard
transmission vs pump power ETPA experiments, presented in many reports, with
our novel approach of transmission vs two-photon temporal delay. Secondly, a
detailed study of the effects of optical losses, unrelated to ETPA, over the
HOM interferogram is carried out by: 1) Characterizing RhB in solutions
prepared with different solvents. 2) Considering scattering losses introduced
by silica nanoparticles used as a controlled linear loss mechanism. Our results
clearly expose the deleterious effects of linear optical losses over the ETPA
signal when standard transmission experiments are employed and show how, by
using the HOM interferogram as a sensing device, it is possible to detect the
presence of such losses. Finally, once we showed that the HOM interferogram
discriminates properly linear losses, our study also reveals that under the
specific experimental conditions considered here, which are the same than those
employed in many reported works, the ETPA was not unequivocally detected.
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