High-fidelity entanglement of polar molecules by dynamic geometric control
- URL: http://arxiv.org/abs/2607.13008v1
- Date: Tue, 14 Jul 2026 17:51:29 GMT
- Title: High-fidelity entanglement of polar molecules by dynamic geometric control
- Abstract summary: We show that by controlling the geometry of the dipolar interaction, even when a molecule occupies many motional states in the tweezer, coherence can be preserved.<n>We characterize several geometries that suppress sensitivity to thermal fluctuations.<n>We further use programmable, coherence-preserving motion of the molecules during entanglement to refocus dephasing from relative positional jitter of the tweezers.
- Score: 1.8658208648963193
- License: http://arxiv.org/licenses/nonexclusive-distrib/1.0/
- Abstract: In quantum information systems made of optical tweezer arrays of ultracold molecules, thermal motion of molecules degrades the coherence of their interactions, which limits entanglement fidelity and the concomitant scientific applicability of these systems. We show that by controlling the geometry of the dipolar interaction, even when a molecule occupies many motional states in the tweezer, coherence can be preserved. We characterize several geometries that suppress sensitivity to thermal fluctuations. We further use programmable, coherence-preserving motion of the molecules during entanglement to refocus dephasing from relative positional jitter of the tweezers, which is relevant even on the 10 nm scale. These methods yield substantially improved dipolar coherence and enable generation of two-molecule entanglement with a Bell state fidelity of $\mathcal{F}= 0.976^{+0.008}_{-0.011}$ in directly laser-cooled molecules.
Related papers
- Ro-vibrational van der Waals interaction between ultracold polar molecules [0.0]
We describe the ro-vibrational van der Waals interaction between ultracold polar molecules.<n>This interaction is strong, leading to fast elastic collisions and orders of magnitude suppression of collisional loss.<n>The scheme is compatible with microwave shielding, where it enables controlled state dependent interactions.
arXiv Detail & Related papers (2026-07-28T14:32:37Z) - Unveiling the Dance of Molecules: Ro-Vibrational Dynamics of Molecules under Intense Illumination at Complex Plasmonic Interfaces [0.0]
The study investigates relaxation dynamics of an ensemble of molecules following intense resonant pump excitation in Fabry-Perot cavities and at three-dimensional plasmonic metasurfaces.<n>The simulations reveal dramatically modified relaxation pathways inside cavities compared to free space, characterized by persistent molecular alignment.<n>They also indicate the presence of a previously unreported relaxation stabilization mechanism driven by dephasing of the collective molecular-cavity mode.
arXiv Detail & Related papers (2024-12-03T22:17:35Z) - Unraveling a cavity induced molecular polarization mechanism from collective vibrational strong coupling [0.0]
We show that collective vibrational strong coupling of molecules in thermal equilibrium can give rise to significant local electronic polarizations in the thermodynamic limit.
Our findings suggest that the thorough understanding of polaritonic chemistry, requires a self-consistent treatment of dressed electronic structure.
arXiv Detail & Related papers (2023-06-09T16:18:51Z) - Quantum Control of Atom-Ion Charge Exchange via Light-induced Conical
Intersections [66.33913750180542]
Conical intersections are crossing points or lines between two or more adiabatic electronic potential energy surfaces.
We predict significant or measurable non-adiabatic effects in an ultracold atom-ion charge-exchange reaction.
In the laser frequency window, where conical interactions are present, the difference in rate coefficients can be as large as $10-9$ cm$3$/s.
arXiv Detail & Related papers (2023-04-15T14:43:21Z) - Dipolar spin-exchange and entanglement between molecules in an optical
tweezer array [0.0]
Ultracold polar molecules are promising candidate qubits for quantum computing.
Using a molecular optical tweezer array, single molecules can be moved and separately addressed for qubit operations.
We demonstrate a two-qubit gate to generate entanglement deterministically, an essential resource for all quantum information applications.
arXiv Detail & Related papers (2022-11-17T18:53:42Z) - Tuning long-range fermion-mediated interactions in cold-atom quantum
simulators [68.8204255655161]
Engineering long-range interactions in cold-atom quantum simulators can lead to exotic quantum many-body behavior.
Here, we propose several tuning knobs, accessible in current experimental platforms, that allow to further control the range and shape of the mediated interactions.
arXiv Detail & Related papers (2022-03-31T13:32:12Z) - High-resolution 'magic'-field spectroscopy on trapped polyatomic
molecules [62.997667081978825]
Rapid progress in cooling and trapping of molecules has enabled first experiments on high resolution spectroscopy of trapped diatomic molecules.
Extending this work to polyatomic molecules provides unique opportunities due to more complex geometries and additional internal degrees of freedom.
arXiv Detail & Related papers (2021-10-21T15:46:17Z) - Evolution of a Non-Hermitian Quantum Single-Molecule Junction at
Constant Temperature [62.997667081978825]
We present a theory for describing non-Hermitian quantum systems embedded in constant-temperature environments.
We find that the combined action of probability losses and thermal fluctuations assists quantum transport through the molecular junction.
arXiv Detail & Related papers (2021-01-21T14:33:34Z) - Magnetic properties and quench dynamics of two interacting ultracold
molecules in a trap [0.0]
We investigate the magnetic properties and nonequilibrium dynamics of two interacting ultracold polar and paramagnetic molecules in a harmonic trap in external electric and magnetic fields.
The molecules interact via a multichannel two-body contact potential, incorporating the short-range anisotropy of intermolecular interactions.
arXiv Detail & Related papers (2020-10-22T17:35:46Z) - Dipolar evaporation of reactive molecules to below the Fermi temperature [2.9989215527241453]
Inelastic losses in molecular collisions have greatly hampered the engineering of low-entropy molecular systems.
Here, we use an external electric field along with optical lattice confinement to create a two-dimensional (2D) Fermi gas of spin-polarized potassium-rubidium (KRb) polar molecules.
Direct thermalization among the molecules in the trap leads to efficient dipolar cooling, yielding a rapid increase in phase-space density.
arXiv Detail & Related papers (2020-07-23T22:02:59Z) - Effects of Conical Intersections on Hyperfine Quenching of Hydroxyl OH
in collision with an ultracold Sr atom [62.60678272919008]
We report on ultracold collision dynamics of the hydroxyl free-radical OH with Sr atoms leading to quenching of OH hyperfine states.
Our quantum-mechanical calculations of this process reveal that quenching is efficient due to anomalous molecular dynamics in the vicinity of the conical intersection.
arXiv Detail & Related papers (2020-06-26T23:27:25Z) - Dynamical Strengthening of Covalent and Non-Covalent Molecular
Interactions by Nuclear Quantum Effects at Finite Temperature [58.999762016297865]
Nuclear quantum effects (NQE) tend to generate delocalized molecular dynamics.
NQE often enhance electronic interactions and, in turn, can result in dynamical molecular stabilization at finite temperature.
Our findings yield new insights into the versatile role of nuclear quantum fluctuations in molecules and materials.
arXiv Detail & Related papers (2020-06-18T14:30:29Z)
This list is automatically generated from the titles and abstracts of the papers in this site.
This site does not guarantee the quality of this site (including all information) and is not responsible for any consequences.